Evaluating uncertainty of some radiation measurand using Monte Carlo method

Nuclear Science and Technology, Vol.9, No. 4 (2019), pp. 34-40  
Evaluating uncertainty of some radiation measurand using  
Monte Carlo method  
Bui Duc Ky*, Nguyen Ngoc Quynh, Duong Duc Thang, Le Ngoc Thiem, Ho Quang Tuan,  
Tran Thanh Ha, Bui Thi Anh Duong, Nguyen Huu Quyet, Duong Van Trieu  
Institute for Nuclear Science and Technology, Hanoi, Vietnam  
(Received 07 November 2019, accepted 26 December 2019)  
Abstract: Evaluating measurement uncertainty of a physical quantity is a mandatory requirement for  
laboratories within the recognition ISO/IEC 17025 certification to access reliability of measured  
results. In this work, the uncertainty of ionizing radiation measurements such as air-kerma, personal  
dose equivalent       was evaluated based on GUM method and Monte Carlo method. An  
uncertainty propagation software has been developed for evaluation of the measurement uncertainty  
more convenient.  
Key words: Uncertainty measurement, Monte Carlo method.  
In this work, uncertainty of air-kerma  
and personal dose equivalent       
quantities were evaluated by both methods.  
These two quantities are the fundamental  
quantities in radiation protection field. All  
experimental data published in this work  
were measured at the Secondary Standard  
Dosimetry Laboratory belongs to Institute for  
Nuclear Science and Technology.  
I. INTRODUCTION  
The measurement uncertainty is a  
characteristic for the dispersion of measurable  
values of a quantity to be measured [1, 2, 3].  
Because without the measurement uncertainty,  
the results of the measurements cannot be  
compared to each other, nor can be compared  
to conventional true values.  
In the field of measurement of ionizing  
radiation ISO/IEC and IAEA has provided  
guidance on measurement uncertainty for  
different measurement quantities. These  
documents are primarily based on the  
evaluation methods provided by the  
International Commission on Measurement  
II. METHODS  
The relationship between a single real  
output quantity y and a number of real input  
quantities   has the following equation (1).  
 
 
 
 
                
    
 
A. GUM method  
Guidelines  
(JCGM).  
The  
uncertainty  
propagation method described in the JCGM  
100:2008 “Guide to the expression of  
uncertainty in measurement” is often referred  
to as the GUM method. The Monte Carlo  
method was described in its supplement 1  
“Guide to the expression of uncertainty in  
measurement – Propagation of distributions  
using a Monte Carlo method”.  
Uncertainty of the input quantities       
 
are divided into two categories, based on how  
its values were evaluated. If it was evaluated  
based on statistical means, they are called type  
A. Otherwise, they are nominated type B.  
However, it is worth mentioning that this  
classification does not affect the uncertainty  
propagation law.  
©2019 Vietnam Atomic Energy Society and Vietnam Atomic Energy Institute  
BUI DUC KY et al.  
The uncertainty of output quantity Y is  
calculated as [2, 3, 4]:  
approximation.  
This  
makes  
calculated  
uncertainty in many cases inaccurate.  
 
    
      
B. Monte Carlo method  
 
 
 
∑
    
          
 
    
 
The Monte Carlo method simulates input  
    
 
∑
∑
    
 
 
         (      )  
 
 
 
 
    
      
quantities   based on initial probability  
 
Where,          and          are  
 
 
 
 
distribution. The distribution of the input  
quantities will affect the output quantity  
according to the model in the equation 1. As  
result, the distribution function of the output  
quantity was obtained. Therefore, not only the  
standard deviation but other characteristics of  
output quantity can be determined (i.e.  
skewness, coverage interval). The process of  
uncertainty evaluation using Monte Carlo  
method was presented in fig.1 [2, 4].  
sensitivity coefficients,           is the  
 
 
estimated covariance associated with   and   .  
 
 
The GUM uncertainty framework  
requires [4]:  
a) The non-linearity of the measurement  
function to be insignificant.  
b) The central limit theorem to apply,  
implying the representativeness of the  
Probability density function (PDF) for the  
output quantity by a Gaussian distribution or a  
t-distribution.  
The advantages of the Monte Carlo  
method are that it doesn’t make any  
assumption about linearity of measurement  
function nor PDF of the output quantity.  
Therefore, the Monte Carlo method is valid for  
wider range of problem compare to GUM  
method. Its result can be used to validate the  
result of GUM method.  
c)  
The  
adequacy  
of  
the  
Welch-  
Satterthwaite formula for calculating the  
effective degrees of freedom.  
In practice, the GUM method is  
frequently used in violation of the requirements  
listed above or without knowing whether these  
requirements hold (with an unquantified degree  
of approximation). Furthermore, the equation 2  
is only the first order Taylor series  
The disadvantage of the Monte Carlo  
method is that it is impossible using hand  
calculation. This method must be implemented  
in a computer software.  
Fig. 1. Uncertainty measurement using a Monte Carlo method for a univariate, real measurement function.[4]  
35  
EVALUATING UNCERTAINTY OF SOME RADIATION MEASURAND USING…  
measurement  
distribution,  
are  
included:  
Gaussian  
Poisson  
C. INST-MC software  
A software program, namely INST-MC  
t-distribution,  
distribution, uniform distribution, triangular  
distribution, etc. The program was validated  
by comparing with the NIST uncertainty  
machine, an uncertainty software has been  
developed by National Institute of Standard  
and Technology/ USA.  
was developed to facilitate the uncertainty  
evaluation. The interface of the software is  
shown in fig.2. Both methods of uncertainty  
evaluation  
discussed  
above  
were  
implemented. In the first version of INST-  
MC, most common distributions in radiation  
INST-MC  
Fig. 2. Interface of INST-MC uncertainty software.  
for the deviation of the actual air pressure P  
III. RADIATION MEASURAND  
from the reference temperature     
 
A. Air-kerma      of 137Cs source.  
    
     mbar,   
corrects for the unstable of  
     
ionization chamber,   
corrects for the  
The air-kerma is obtained from Eq.3  
    
possible deviation of the actual distance of the  
reference source to the measuring instrument  
from the nominal calibration distance.  
 
    
        
    
    
 
      
 
Where:   is calibration factor of  
 
ionization chamber,   is correction factor of  
Using the equation 2, uncertainty of air-  
kerma U(K) and corrected reading U(Mcorr) is  
given by:  
 
the difference between the reference beam  
quality,  , and the actual quality,  , during the  
 
measurement and   
ionization chamber:  
is corrected reading of  
      
      
     
      
    
 
      
 
 
 
 
 
 
 
      
      
 
    
√
 
 
 
 
      
 
 
 
      
              
                       
    
    
 
      
 
      
 
is reading of ionization chamber,  
    
 
 
 
 
 
 
 
 
 
 
 
 
 
    
 
    
    
    
 
 
 
(
)   (  
)   (  
)
    
 
corrects for the deviation of the actual  
 
 
 
 
 
    
 
 
 
 
  
  
    
 
 
 
 
 
 
      
    
    
    
 
air temperature  
T
from the reference  
     
    
 
 
 
  (  
)
    
    (  
)
 
 
 
    
 
 
     
      
√
temperature            K,     
corrects  
 
 
 
36  
BUI DUC KY et al.  
corrects for the inhomogeneity response of  
dosimeter,   corrects for others affect.  
B. Personal dose equivalent       using  
TLD dosimeter.  
      
Personal dose equivalent Hp(d) is  
The uncertainty of personal dose  
obtained from equation (7):  
equivalent     ) is obtained from equation 10.  
               
 
    
      
        
 
    
 
                  
          
 
    
      
 
Where: M is reading of exposed dosimeter,   
is reading of background dosimeter.  
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
        
       
 
(
)   (  
)   
      
     
 
 
ECC is elements correction coefficients.  
 
 
    
    
 
      
 
 
     
(
)   (  
)   
    
 
 
 
̅
 
 
 
      
    
 
 
    
 (  
)
    
      
    
    
 
 
(
)   (  
)   (  
)
 
 
    
 
      
    
√
̅
  is average reading of n dosimeters and   is  
 
th  
̅̅̅̅̅̅̅  
IV. RESULTS AND DICUSSION  
reading of i dosimeter (i=       ).  
RCF is reader calibration factor:  
A. Uncertainty of air-kerma with the  
gamma rays of 137Cs.  
      
 
      
    
 
 
The measurement uncertainty of air-  
C is reading of calibration set,   is reading of  
 
kerma   
using approximation method  
     
background calibration set,   is conventional  
 
estimated around 1.26%. The uncertainty  
corresponds to a coverage factor k = 1 and a  
level of confidence factor of approximately p =  
68%. The details of uncertainty of components  
showed in Table I.  
true value (exposed dose),   corrects for  
 
energy dependence of dosimeter,   corrects  
    
for non-linearity of dosimeter,   corrects for  
 
the loss signal before reading dosimeter,   
    
Table I. Uncertainty budget of air-kerma  
Relative standard  
deviation (%)  
Type of  
uncertainty  
Degree of  
freedom  
Source of uncertainty  
Calibration factor of ionization  
chamber  
0.41  
B
-
Reading of ionization chamber  
Air pressure  
0.10  
0.11  
0.10  
0.13  
0.60  
1.00  
A
B
9
-
-
-
-
-
Air temperature  
B
Distance  
B
Stability of ionization chamber  
Others  
A, B  
A, B  
 
 
1.26  
37  
EVALUATING UNCERTAINTY OF SOME RADIATION MEASURAND USING…  
Calculation model of air-kerma  
using INST-MC software is given by  
equation (11):  
Based on data in table III, Monte Carlo  
method estimated measurement uncertainty of  
air-kerma approximately 1.21% correspond a  
coverage factor k = 1 and a level of confidence  
factor of approximately p = 68%.  
 
                        
         
     
    
 
    
 
 
Table II. Distribution of input quantities of air- kerma  
Average value  
Standard  
deviation  
Degree of  
freedom  
Input quantities,   
Distribution  
Student  
 
of   
 
Reading of ionization chamber,  
4.175  
50.23  
0.035  
0.27  
3
3
 
    
Calibration factor of ionization  
Student  
chamber,   
 
 
0.997  
1.008  
1.001  
0.999  
0.007  
Rectangular  
Rectangular  
Constant  
-
-
-
-
 
 
 
0.0006  
 
     
-
-
 
    
Rectangular  
Figure 3 show the detail of the  
close. That means GUM method is valid,  
and uncertainty of air-kerma can be  
calculated by either GUM method or  
Monte Carlo method.  
uncertainty result of air-kerma using  
Monte Carlo method. The uncertainty  
evaluation results of two method are very  
Fig. 3. Measurement uncertainty result of air kerma using INST-MC software  
uncertainty corresponds to a coverage factor  
k = 1 and a level of confidence factor of  
approximately p = 68%. The details of  
uncertainty of components are showed in  
Table III.  
B. Uncertainty of dose equivalent       
using TLD dosimeters.  
The measurement uncertainty of dose  
equivalent  
 
      
using approximation  
method estimated around 18.1%. The  
38  
BUI DUC KY et al.  
Table III. Uncertainty budget of dose equivalent       
Relative standard  
deviation (%)  
Type of  
uncertainty  
Degree of  
freedom  
Source of uncertainty  
Conventional true value (exposed dose), Hc  
Reading of dosimeters, M  
2.36  
2.7  
B
A
-
4
99  
9
-
Elements Correction Coefficients, ECC  
Reader Calibration Factor, RCF  
2.1  
A
3.5  
A, B  
B
 
 
12.6  
6.5  
 
    
B
-
 
    
9.1  
B
-
 
1.9  
3.0  
B
-
-
 
others  
-
 
 
18.1  
Calculation model of dose equivalent  
      is given by equation (7). Based on  
distribution of input quantities of personal dose  
equivalent        in table IV, INST-MC  
estimated measurement uncertainty of dose  
equivalent approximately 18.7% correspond a  
coverage factor k = 1 and a level of confidence  
factor of approximately p = 68%. Fig.4 show  
the detail of uncertainty of personal dose  
equivalent Hp(d) using Monte Carlo method.  
Table IV. Distribution of input quantities of personal dose equivalent        
Standard  
deviation  
Degree of  
freedom  
Input quantities,   
Value of   
Distribution  
 
 
Reading of dosimeter,       
4817  
0.88  
15443  
6.8  
90.48  
0.07  
Student  
Student  
5
99  
5
7
-
 
Elements Correction Coefficients, ECC  
Reading of calibration set,       
545  
Student  
 
Conventional true value,   
0.082  
0.08  
Student  
 
0.615  
1.02  
1.02  
0.98  
Rectangular  
Rectangular  
Rectangular  
Rectangular  
 
 
0.034  
0.091  
0.019  
-
 
    
 
    
-
-
 
 
39  
EVALUATING UNCERTAINTY OF SOME RADIATION MEASURAND USING…  
Fig. 4. Measurement uncertainty result of     ) using INST-MC software  
IV. CONCLUSIONS  
[4]. NPL report MS6 - Software support for  
metrology – Uncertainty evaluation, M G  
The measurement uncertainty of air-  
Cox and P M Harris, National Physical  
kerma and the personal dose equivalent       
 
Laboratory, march 2010.  
were evaluated by the GUM method and  
[5]. On a Monte Carlo method for measurement  
Monte  
Carlo  
method,  
which  
were  
uncertainty  
evaluation  
and  
its  
implemented in the INST-MC software  
program. The results showed that deviations  
of air-kerma and personal dose equivalent  
       calculated by two methods are 3.9%  
and 3.3%, respectively. Compared with the  
approximation method, INST-MC is more  
convenient to calculate and it also shows the  
probability distribution of the obtained results.  
implementation, P M Harris and M G Cox,  
Metrologia 51, 2014.  
[6]. Uncertainty analysis of phase and amplitude of  
harmonic components of bearing inner ring  
four-point roundness measurement, Raine  
Viitala et al, Precision Engineering, 2018.  
[7]. Estimation of uncertainty of effective area of a  
pneumatic pressure reference standard using  
Monte Carlo method, Singh et al, Indian  
Journal of Pure & Applied Physics, 2016.  
In  
further  
research,  
uncertainty  
evaluation of other quantities in SSDL will be  
estimated by Monte Carlo method.  
[8]. A Guide on Measurement Uncertainty in  
Medical Testing, Technical Guide 4, the  
Singapore Accreditation Council, 2013.  
RERERENCES  
[1]. ISO 17025:2005, General requirements for  
the competence of testing and calibration  
laboratories.  
[9]. Calibration of radiation protection and  
monitoring instrument, IAEA safety report  
series No.16, 2000.  
[2]. Evaluation of measurement data – Guide to the  
expression of uncertainty in measurement,  
JCGM 100:2008, 2008.  
[10]. Evaluation of measurement data  
–
Supplement 1 to the "Guide to the expression  
of uncertainty in measurement" – Propagation  
of distributions using a Monte Carlo method,  
JCGM 101:2008, 2008.  
[3]. Revision of the Guide to Expression of  
Uncertainty in Measurement, Walter Bich et  
al, Metrologia, 49, 2012.  
40  
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