Development of neutron survey meter using prescila neutron probe

Nuclear Science and Technology, Vol.8, No. 4 (2018), pp. 26-33  
Development of neutron survey meter  
using prescila neutron probe  
1,*  
1
 
 
Luong Thi Hong , Nguyen Tien Phong , Pham Thi Bich , Nguyen Duc Huyen  
1 Center for Non – Destructive Evaluation; 140 Nguyen Tuan, Thanh Xuan, Hanoi, Vietnam  
* Corresponding email: [email protected]  
(Received 20 December 2018, accepted 20 February 2019)  
Abstract: This paper presents the design and validation of a neutron survey meter. The meter consists  
of a PRESCILA neutron probe (with good sensitivity, directional response, gamma rejection, and  
enhanced high-energy response to 20 MeV) and an electrometer developed at Non-Destructive  
Evaluation center. The homogeneity response of the PRESCILA neutron probe was investigated as a  
    
 
function of distances from the  
        source in order to obtain the appropriate distance for  
accurate count-rate measurements using the neutron survey meter. A system consists of the  
PRESCILA neutron probe and the Ludlum Model 2326 electrometer was then used for measuring  
neutron ambient dose equivalent rates in the range from 50 cm to 200 cm with the step of 25 cm. The  
relationship between the count-rates and neutron dose equivalent rates (in the distance ranged from 50  
to 200 cm) were deduced to validate the proper operation of the neutron survey meter.  
Keywords: Neutron survey meter, PRESCILA neutron probe, Ludlum electrometer.  
MeV), high sensitivity, and moderate gamma  
rejection [1].  
I. INTRODUCTION  
A
neutron survey meter normally  
This paper presents the fabrication of a  
neutron survey meter for the purpose of safety  
assessment, which consists of a set of five  
PRESCILA neutron probes and a self-  
developed electrometer designed by Non-  
Destructive Evaluation (NDE) center. The  
validation of proper operation of the survey  
meter was also investigated using the neutron  
standard fields at the Institute for Nuclear  
Science and Technology (INST) [2,3].  
constitutes of an electrometer and a single or  
multiple neutron detectors. Principle of a  
conventional neutron survey meter is based on  
1960s technology that relies on a large neutron  
moderator assembly surrounding a thermal  
detector to achieve a response function over a  
limited energy range. Such neutron survey  
meter reveals an ergonomic challenge, being  
heavy and bulky, and have caused injuries  
during radiation protection surveys [1].  
Another defect of the traditional neutron  
survey meter is a poor high-energy response  
above 10 MeV, which makes them unsuitable  
for neutron dose measurements at high-energy  
neutron facilities (i.e. medical linear  
accelerators). The PRESCILA Proton Recoil  
Scintillator developed Los Alamos National  
Laboratory is a light-weight (2 kg) probe with  
extended high-energy response (up to 20  
II. MATERIAL AND METHOD  
A. PRESCILA neutron probe  
The model 42-41L PRESCILA neutron  
probe was developed by the Health, Safety, and  
Radiation Protection Division at the Los Alamos  
National Laboratory. The probe is the  
combination of a dual-scintillator ZnS(Ag)+6LiF  
and ZnS(Ag) + plastic, using both fast and  
©2018 Vietnam Atomic Energy Society and Vietnam Atomic Energy Institute  
LUONG THI HONG et al.  
thermal neutron detectors, made it possible to  
The 3D view of the PRESCILA probe is  
shown in Fig.(1a) and the structure is shown in  
Fig.(1b). Where, “11” is a light guide; “11a” is  
the central penetration beamline; “12-13-14” are  
the top, bottom, and the side plates with 5%  
borated polyethylene, respectively; “12a” is a  
central aperture; “15” is central apertures for  
insertion of fast neutron scintillators  
(ZnS(Ag)+plastic); “16” is a cadmium (Cd)  
filter; “17” is a thermal neutron scintillator  
(ZnS(Ag)+6LiF); “18” is a plastic spacer; 19 is  
a photomultiplier tube (PMT) and “20” is a  
handle [4].  
balance the overall energy response and provide  
adequate response in the crossover region  
between the thermal and fast neutron energy.  
The probe is capable of excellent  
sensitivity (40 counts per minute per μSvh-1 for  
241Am-Be source) and extended high-energy  
response up to 20 MeV. The directional  
response is uniform within 15% over a wide  
range of energy. The linearity response has  
been confirmed up to a dose rate of 20 mSvh-1.  
The probe has high-dose gamma rejection up  
to 2 mSv.h-1 [1].  
(a): 3D outer view  
(b): different components  
Fig. 1: PRESCILA (Model 42-41L) neutron probe [4].  
The fast neutrons are detected using a  
powders on the back of a Lucite disc. The  
thermal neutrons are detected via the  
phosphor scintillator of ZnS(Ag) powder via  
 
 
(
)
proton recoil process. The blue light        
  (n,α)   reactions [5].  
as the result of scintilation process is then  
recorded by a photomultiplier tube. The  
detection process can be expressed as  
follows555 [5]:  
B. Commercial neutron survey meter  
A commercial gamma/neutron survey  
meter including a model 2363 Ludlum  
electrometer and the model 42-41L  
PRESCILA neutron probe was used to measure  
neutron dose equivalent rates at various  
distances from the source. The measured  
values were then used to compare with the data  
measured using the developed neutron meter.  
 
(
)[  
]
(
)
                           
(
)
                     
Thermal and epithermal neutrons are  
detected using a thermal scintillator (Eljen EJ-  
 
420P) which is a mixture of   F and ZnS(Ag)  
27  
DEVELOPMENT OF NEUTRON SURVEY METER USING PRESCILA NEUTRON PROBE  
The commercial neutron survey meter  
has an energy-compensated GM (allowing  
gamma detection) and a neutron detector based  
on proton recoil scintillation process. The  
meter is significantly lighter than other  
traditional neutron survey meter. Fig. 2 shows  
the commercial neutron survey meter [1].  
C. Electrometer designed by NDE  
In this paper, an electrometer  
developed by NDE is presented, which is  
constituted of an analog electronic block of  
different components such as high voltage  
power supply, pre-amplifier, pulse shapper,  
real time clock module, counter timer, etc.  
The microprocessor-based central processing  
unit controls the counting, calculating,  
displaying of results on a graphic LCD  
monitor, etc. The electrometer console is  
user-friendly interface. Pulse discrimination  
was accounted into the electronic block for  
gamma rejection. This electrometer was then  
connected to the model 42-41L PRESCILA  
neutron probe to constitute a neutron survey  
meter. The electronic diagram of the neutron  
meter is shown in Fig. 3.  
Fig. 2. Commercial neutron survey meter consists  
of a model 2326 Ludlum electrometer and a  
model 42-41L PRESCILA neutron probe [5].  
Fig. 3. Neutron survey meter consists of a commercial model 42-41L PRESCILA neutron probe and an  
electrometer designed at NDE (the component inside the dashed line).  
28  
LUONG THI HONG et al.  
The design goal of neutron survey meter  
being optimized in a wide energy range [1]. In  
this section, the investigation of the effective  
distance of the self-developed neutron survey  
meter for measurements is performed.  
Therefore, the count rates obtained by the self-  
developed neutron survey meter exposed to 02  
bare 241Am-Be neutron sources (80 mCi and 40  
mCi) were recorded and analyzed. In this  
experiment, two neutron sources were placed  
at the distance range from 0 cm to 75 cm (with  
a step of 15 cm) from the detector surface. The  
experimental setup can be seen in Fig. 4. The  
total count rates measured by the self-  
developed neutron survey meter are tabled in  
Table I (each value is averaged over 05  
measurements).  
is to balance the under response in the range  
from about 0.1 MeV to 2 MeV by an over  
response below 0.1 MeV that would give the  
most accurate results for a range of practical  
field spectra, with the applied radiation  
weighting factor (WR =10), so when the  
calibration of the dose rates is much simpler  
(usually using the energy of the neutron  
emitted by 241Am-Be or 252Cf). More detailed  
characteristics of neutron probe used in the  
neutron survey meter developed by NDE can  
be found in the manufacturer’s specifications  
[5]. A combination of lead and cadmium  
filters is assembled with the scintillator probe.  
The lead filter (2.84 cm in diameter, 0.038 cm  
in thickness) is used to reduce the  
scintillator’s sensitivity to low-energy  
photons, while the cadmium filter (1.91 cm in  
diameter, 0.039 cm in thickness) is used to  
reduce the thermal neutron response below the  
cadmium cut-off energy.  
Model 42-41L  
Electrometer  
PRESCILA  
neutron probe  
designed by NDE  
III. RESULT AND DISCUSSION  
02 bare 241Am-Be  
neutron sources (80  
and 40 mCi)  
A. Effective distance of the self-developed  
neutron survey meter  
The use of both fast and thermal  
scintillator allows the energy response function  
of the self-developed neutron survey meter  
Fig. 4. Experimental setup for investigating the  
effective distance.  
Table I. The count rates (cpm) measured by the self-developed neutron survey meter at various distances  
from the two neutron sources.  
Electrometer  
designed by NDE  
Center  
Side I  
Side II  
Side III  
D
(cm)  
Count  
rate  
Count  
rate  
Count  
rate  
Count  
rate  
Count  
rate  
A
SD  
P (%)  
(cpm)  
(cpm)  
(cpm)  
(cpm)  
(cpm)  
0
1106.2  
342.8  
188.2  
1512.0  
399.0  
197.0  
1447.4  
394.8  
202.6  
1473.6  
413.8  
209.6  
1616.0  
416.8  
217.0  
1431.0  
393.4  
202.9  
180.9  
31.5  
14.9  
60.0  
70.0  
90.0  
15  
30  
29  
DEVELOPMENT OF NEUTRON SURVEY METER USING PRESCILA NEUTRON PROBE  
45  
60  
75  
117.8  
83.8  
61.8  
131.2  
87.6  
64.0  
121.8  
86.0  
62.4  
130.4  
88.8  
63.8  
135.8  
88.8  
62.8  
127.4  
87.0  
63.0  
14.5  
6.6  
95.0  
99.0  
99.5  
5.4  
-
P is the detection probability which is a function of distance from the source (probability as  
Confidence intervals of value average with each distance);  
D is distance from source to detector;  
-
-
-
-
-
Side I, II, III, IV is four sides with fast scintillators;  
Center is the side with thermal scintillator;  
SD is standard deviation;  
A is the count rates averaged over all of five sides.  
The effective distance for the  
laboratory at INST. The count rate measured  
by the self-developed neutron survey meter in  
each of five sides (4 thermal sides and one  
central fast side) of the neutron probe were  
performed. The measurements were performed  
at three distances of 50cm, 75cm and 100cm.  
The data were collected for X-Y planes and  
shown in 360º of Z plane (angle from 0º to  
360º with a step of 30º). The results are  
presented in Fig. 5 (0o at the top position). The  
measured values show the maximum deviation  
of about 14% over 360o responses.  
measurements using the self-developed neutron  
survey meter was chosen at the distances that  
the “P” values greater than 95%. From Table 1,  
it implies that the measurements should be  
conducted at a distance more than 45 cm from  
the source.  
B. Angular dependence of the self-developed  
neutron survey meter  
The angular dependence of the self-  
developed neutron survey meter was  
investigated at the secondary standard dosimetry  
1201  
629  
386  
1203  
541  
1512  
573  
348  
346  
329  
377  
517  
1184  
554  
1139  
SDD100  
Fig. 5. Homogeneity response of the self-developed neutron survey meter at various angles.  
30  
LUONG THI HONG et al.  
In order to verify the accuracy of the  
C. Validation of the self-developed neutron  
survey meter  
self-developed neutron survey meter, the meter  
was calibrated at the secondary standard  
dosimetry laboratory at the INST. The total  
neutron ambient dose equivalent rates (unit in  
µSv.h-1) were measured at distances from 60 to  
150 cm in the standard neutron field of a bare  
241Am-Be source. The response due to the  
direct component of neutron field was then  
analyzed and compared with the reference  
values reported in Refs. [2, 3] to confirm the  
proper operation of the self-developed neutron  
survey meter. The results are shown in Table 2.  
Once the effective distance from the  
source to the detector was obtained for the self-  
developed neutron survey meter, the neutron  
ambient dose equivalent rates were measured  
using the commercial neutron survey meter in  
the distance range from 50 cm to 150 cm. The  
total count rates were also measured using the  
self-developed neutron survey meter in the  
same distance range from 50 cm to 150 cm  
with the step of 25 cm. The total count rates  
were then fitted as a function of the neutron  
dose equivalent rates (measured using the  
commercial neutron survey meter). The  
relationship is shown in Fig. 6 and used to  
compute the displayed function of the self-  
developed neutron survey meter (i.e. display  
unit of the self-developed neutron survey meter  
is functioned in µSv.h-1).  
From Table II, ones can see that the  
neutron ambient dose equivalent rates  
measured by the NDE center self-developed  
neutron survey meter and those in the free  
field are in good agreement within 1% . This  
means that the self-developed neutron survey  
meter can be well applied in the practical  
neutron ambient dose equivalent rate  
measurements.  
Fig. 6. Neutron ambient dose equivalent rates (μSv/h in Y axis, measured by a commercial neutron survey meter)  
as a function of the total count rates (cpm in X axis, measured by the self-developed neutron survey meter).  
31  
DEVELOPMENT OF NEUTRON SURVEY METER USING PRESCILA NEUTRON PROBE  
Table II. The neutron ambient dose equivalent rates (due to the direct component of a neutron standard field  
of a bare 241Am-Be source) measured by the self- developed neutron survey meter in the comparison  
with the standard ones.  
Ambient dose equivalent rates  
Standard ambient dose  
Distance  
(cm)  
measured by the self- developed  
neutron survey meter  
(μSv/h)  
Deviation  
(%)  
equivalent rates  
(μSv/h)  
60  
70  
402  
295  
226  
145  
101  
64  
400  
294  
225  
144  
100  
64  
0.49  
0.37  
0.43  
0.68  
0.98  
0.00  
80  
100  
120  
150  
V. CONCLUSIONS  
ACKNOWLEDGEMENT  
In this work, the neutron survey meter  
was introduced based on the commercial  
neutron probe (model 42-41L PRESCILA)  
and a self-developed electrometer by NDE.  
The effective distance for the measurements  
using the meter was investigated. The other  
characteristics of the neutron survey meter  
were also evaluated, such as the  
homogeneity response, the dose equivalent  
rate response. Moreover, the neutron survey  
meter was also calibrated at the secondary  
standard dosimetry laboratory at the  
This work has been financially  
supported by the Vietnam Ministry of Science  
and  
Technology  
under  
the  
project  
The  
ĐTCB.02/17/TTNDE  
(2017-2018).  
authors would like to thank Dr. Le Ngoc  
Thiem, MSc. Nguyen Ngoc Quynh and Ms.  
Dang Thi My Linh at INST for their valuable  
comments during the manuscript preparation.  
REFERENCES  
[1]. Richard H. Olsher, David T. Seagraves,  
Shawna L. Eisele, Christopher W. Bjork,  
William A. Martinez, Leonard L. Romero,  
Michael W. Mallett, Michael A. Duran,†and  
Institute  
for  
Nuclear  
Science  
and  
Charles R. Hurlbut; “Prescila:  
A
new  
Technology in order to confirm the proper  
operation. In the future, other characteristics  
of the neutron meter (dose range sensitivity,  
energy range response, gamma rejection,  
etc) will be verified to reconfirm the  
practical funtionality in neutron safety  
assessment.  
lightweight neutron rem meter”; Health  
Physics, Volume 86, Number 6, June 2004.  
[2]. Le Ngoc Thiem et al.; “Characterization of a  
Neutron Calibration Field with 241Am − Be  
Source using Bonner Sphere Spectrometer”;  
Applied Radiation and Isotopes; Vol. 133, pp.  
68-74, 2018.  
32  
LUONG THI HONG et al.  
[3]. Le Ngoc Thiem et al.; “Neutron Calibration  
Field at Institute for Nuclear Science and  
Technology”; Nuclear Science and  
Technology, Vol.6, No. 4, pp. 01-07, 2016.  
[5]. Serial Number 220855 and Succeeding Serial  
Numbers, “Ludlum Model 2363 Gamma-  
Neutron  
Survey  
Meter”,  
Ludlum  
Measurements, INC, 2015. ICRP. “Conversion  
Coefficients for use in Radiological Protection  
against External Radiation”, ICRP Publication  
74. Ann. ICRP 26 (3-4), 1996.  
[4]. Richard H. Olsher, Los Alamos, NM (US); et al.:  
“Proton recoil Scintillator Neutron Rem meter”;  
United States Patent Application Publication Pub.  
No.: US2002/0141529 A1; Oct.3, 2002.  
33  
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